We present a search for like-sign dielectrons plus multijet events using 107 pb^-1 of data in ppbar collisions at sqrt s = 1.8 TeV collected in 1992-95 by the CDF experiment. Finding no events that pass our selection, we set sigma . Br limits on two SUSY processes that can produce this experimental signature: gluino-gluino or squark-antisquark production with R-parity violating decays of the charm squark or lightest neutralino via a non-zero gamma'_121 coupling. We compare our results to NLO calculations for gluino and squark production cross sections and set lower limits on M(~g), M(~t_1), and M(~q).